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null (Ed.)Abstract. In response to the coronavirus disease of 2019 (COVID-19),California issued statewide stay-at-home orders, bringing about abrupt anddramatic reductions in air pollutant emissions. This crisis offers us anunprecedented opportunity to evaluate the effectiveness of emissionreductions in terms of air quality. Here we use the Weather Research and Forecastingmodel with Chemistry (WRF-Chem) in combination with surface observations tostudy the impact of the COVID-19 lockdown measures on air quality insouthern California. Based on activity level statistics and satelliteobservations, we estimate the sectoral emission changes during the lockdown.Due to the reduced emissions, the population-weighted concentrations of fineparticulate matter (PM2.5) decrease by 15 % in southernCalifornia. The emission reductions contribute 68 % of the PM2.5concentration decrease before and after the lockdown, while meteorologyvariations contribute the remaining 32 %. Among all chemical compositions,the PM2.5 concentration decrease due to emission reductions isdominated by nitrate and primary components. For O3 concentrations, theemission reductions cause a decrease in rural areas but an increase in urbanareas; the increase can be offset by a 70 % emission reduction inanthropogenic volatile organic compounds (VOCs). These findings suggest thata strengthened control on primary PM2.5 emissions and a well-balancedcontrol on nitrogen oxides and VOC emissions are needed to effectively andsustainably alleviate PM2.5 and O3 pollution in southernCalifornia.more » « less
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Abstract. For the radiative impact of individual climate forcings,most previous studies focused on the global mean values at the top of theatmosphere (TOA), and less attention has been paid to surface processes,especially for black carbon (BC) aerosols. In this study, the surface radiativeresponses to five different forcing agents were analyzed by using idealizedmodel simulations. Our analyses reveal that for greenhouse gases, solarirradiance, and scattering aerosols, the surface temperature changes aremainly dictated by the changes of surface radiative heating, but for BC,surface energy redistribution between different components plays a morecrucial role. Globally, when a unit BC forcing is imposed at TOA, the netshortwave radiation at the surface decreases by -5.87±0.67 W m−2 (W m−2)−1 (averaged over global land without Antarctica), which ispartially offset by increased downward longwave radiation (2.32±0.38 W m−2 (W m−2)−1 from the warmer atmosphere, causing a netdecrease in the incoming downward surface radiation of -3.56±0.60 W m−2 (W m−2)−1. Despite a reduction in the downward radiationenergy, the surface air temperature still increases by 0.25±0.08 Kbecause of less efficient energy dissipation, manifested by reduced surfacesensible (-2.88±0.43 W m−2 (W m−2)−1) and latent heat flux(-1.54±0.27 W m−2 (W m−2)−1), as well as a decrease inBowen ratio (-0.20±0.07 (W m−2)−1). Such reductions of turbulentfluxes can be largely explained by enhanced air stability (0.07±0.02 K (W m−2)−1), measured as the difference of the potential temperaturebetween 925 hPa and surface, and reduced surface wind speed (-0.05±0.01 m s−1 (W m−2)−1). The enhanced stability is due to the fasteratmospheric warming relative to the surface, whereas the reduced wind speedcan be partially explained by enhanced stability and reduced Equator-to-poleatmospheric temperature gradient. These rapid adjustments under BC forcingoccur in the lower atmosphere and propagate downward to influence thesurface energy redistribution and thus surface temperature response, whichis not observed under greenhouse gases or scattering aerosols. Our studyprovides new insights into the impact of absorbing aerosols on surfaceenergy balance and surface temperature response.more » « less
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